Quantum transport in nanostructures, quantum dots, molecular electronics, graphene and 2D materials.
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We investigate Floquet-driven topological phase transitions in an AB-stacked bilayer Haldane lattice with tunable intralayer hopping anisotropy. By combining interlayer hybridization, Haldane flux, and off-resonant circularly polarized light, we obtain controlled transitions among Dirac, semi-Dirac, and higher-Chern insulating phases. As the hopping anisotropy increases, the two inequivalent Dirac points move toward each other and merge at the Brillouin-zone $\mathbf{M}$ point, where a semi-Dirac dispersion emerges with linear and quadratic momentum dependence along orthogonal directions. In this regime, competition between the intrinsic Haldane mass and the Floquet-induced mass drives a sequence of sharp topological transitions with Chern numbers $C=0,\pm1,\pm2$. We further show that interlayer coupling qualitatively reshapes the Floquet band topology by inducing helicity-dependent and valley-selective band inversions at the K and K$'$ points, thereby stabilizing higher-Chern phases in the valence bands. These changes are accompanied by redistribution of the Berry curvature, bulk gap closings, and the collapse or sign reversal of quantized anomalous Hall plateaus. As the system approaches the semi-Dirac limit, the topological phase space narrows and disappears at the critical merger point, beyond which the system becomes topologically trivial even when it remains gapped. Overall, the bilayer geometry broadens the scope of Floquet topological control by enabling dynamically tunable higher-Chern phases and valley-dependent Hall responses governed by interlayer coupling and light helicity.
We investigate the impact of an induced mass term $Δ$ on the current density in graphene subjected to a space- and time-dependent periodic potential $U(x,t)$. By solving the Dirac equation and deriving both the quasi-energy spectrum and the corresponding eigenspinors, we obtain explicit analytical expressions for the current density, which exhibits a clear dependence on $Δ$. We show that $Δ$ acts as a tunable control parameter that governs the amplitude, sign, and resonance structure of Josephson-like current oscillations. For normal incidence and a purely time-periodic potential, our results reveal that the oscillations within the energy gap gradually diminish as the mass term $Δ$ increases. This suppression leads to a weakening of the Josephson-like effect typically observed in such systems. When the potential $U(x,t)$ is periodic in both space and time, the behavior becomes more complex. The current density can take either positive or negative values depending on the magnitude of the induced gap, and it generally decreases over time. As a result, the resonance phenomena--prominent at lower gap values--become progressively less significant as $Δ$ increases. These findings underscore the tunable nature of light-matter interactions and quantum transport in gapped graphene, suggesting potential applications in terahertz (THz) nanoelectronic devices and optically controlled quantum switches.
We develop a theory of polarized photoluminescence of interface excitons localized at lateral heterojunctions between transition metal dichalcogenide monolayers. We show that the circular selection rules governing interband optical transitions exactly at the band extrema are modified at finite wave vectors. The corresponding wave-vector-dependent corrections to the optical matrix elements result in a net linear polarization of excitonic photoluminescence. We identify two microscopic mechanisms responsible for linear polarization$-$trigonal warping of the electron and hole dispersions and the energy dependence of the effective masses. Their interplay controls both the magnitude and the angle of the emitted light polarization, with distinct dependences on the crystallographic orientation of the interface. Using a microscopic variational approach, we demonstrate that the degree of linear polarization can reach values exceeding 10% in realistic heterostructures. Furthermore, due to the large built-in dipole moment of interface excitons, their optical response can be tuned by an external in-plane electric field, enabling control over the strength and direction of the polarization.
We investigate topological phase transitions for the Haldane and Kane-Mele model in a lattice with $p6$ symmetry, which consists of triangles and hexagons arranged in a two-dimensional geometry. For the Haldane model, which breaks time-reversal symmetry, we calculate the Chern number using a multi-band non-Abelian Wilson loop formalism. By varying the hopping parameters in the triangles and hexagons independently, a large variety of topological phases emerge. In the presence of a next-next-nearest neighbor hopping, the phase diagram becomes even richer, with regions exhibiting high Chern numbers. Then, we consider the Kane-Mele model, for which time-reversal symmetry is preserved, and calculate the number of $π$-crossings in the Concentric Wilson Loop Spectrum (CWLS). This method is appropriate to determine the topological invariant for systems hosting time-reversal and rotational symmetry, but lacking all other symmetries. According to a classification based on $K$-theory, the CWLS invariant reveals topological properties even when more conventional invariants fail to detect them. The formalism was previously successfully applied to systems with 3- and 4-fold symmetry. Here, we surprisingly find that for the 6-fold-symmetry model investigated, the topology identified by this invariant is fragile, therefore questioning the claim that this should be the strong invariant missing in a complete classification of topological insulators.
Spin-phonon interactions have a dual role in emerging spin-based quantum technologies. While they can be a limitation to device performance through decoherence, they also serve as a critical resource for coherent spin control, detection, and the realization of spin-based quantum networks. However, their direct characterization remains a challenge and is usually material-dependent. Here, we introduce a technique to probe spin-phonon coupling at millikelvin temperatures and gigahertz frequencies, using high-overtone bulk acoustic wave resonators (HBARs) integrated with arbitrary crystals via visco-elastic transfer of thin-film lithium niobate transducers. By tuning the Larmor frequency of dilute spin ensembles into resonance with HBAR modes, we extract the anisotropy and strength of spin-phonon interactions from acoustic dispersion and dissipation measurements. We demonstrate this approach in calcium tungstate (CaWO4) and yttrium orthosilicate (Y2SiO5), achieving cooperativities up to 0.5 for erbium dopant ensembles. Our method enables the study of spin-phonon interactions in complex crystalline materials, with minimal fabrication constraints. These results will facilitate the design of hybrid quantum systems and the quest for ion-matrix combination with enhanced spin-phonon coupling.
We present topological insulator (TI)-based single-electron transistors (SETs) as magnetic-field-compatible charge sensing devices that are easily integrable with TI-superconductor hybrid platforms. We observe well-resolved Coulomb diamonds in the charge-stability diagrams of our devices confirming the charge quantization and single-electron transport. In some devices, the Coulomb resonances show persistent shifts corresponding up to $\sim$ e/2 charge. An axial magnetic field further displaces these shifts to higher or lower gate voltages. We find that the axial magnetic-field dependence of the shifts is consistent with the Zeeman shift of a trap state coupled to the SET, and we reproduce the observations using numerical simulations. The resonance shifts are therefore identified as a consequence of the sensitivity of our TI-SET devices to charges in proximity. Establishing this charge sensing capability is a first step toward integrating TI-SETs as charge sensors in more complex TI-based hybrid devices, with the overarching goal of detecting and braiding Majorana zero modes.
We investigate spin-wave modes in confined ferromagnetic resonators with spherical and cylindrical geometries across the exchange-dominated, dipole-exchange, and dipolar interaction regimes. Starting from the linearized Landau-Lifshitz-Gilbert equation, we show that the projection of the total angular momentum and mirror parity are conserved quantities in the problem of axially symmetric resonators. These symmetries provide a natural classification of spin-wave modes and explain the degeneracy of exchange modes, as well as its lifting by dipolar interactions. Numerical analysis shows that the nonlocal dipolar interaction removes the exchange degeneracy and hybridizes modes, leading to avoided crossings between modes that belong to the same symmetry sector. To describe this behavior, we develop a coupled-mode theory formulated directly in terms of dynamical magnetization, which reduces the dipole-exchange problem to a finite system of interacting modes. The resulting framework provides a unified description of spin-wave spectra in confined magnetic particles from the exchange limit to the dipolar regime.
Generating stable magnetic skyrmions is essential for the practical application of skyrmion-based spintronic devices in thermally agitating environments. Recent advancements have enabled the creation of skyrmions by controlling stripe domain instability through dynamic magnetic-field control. However, deterministic skyrmion creation and effectively managing the thermal stability of skyrmions remain challenges. Here, we present a deep reinforcement learning (DRL) approach to identify advanced dynamic magnetic-field-temperature paths that create skyrmions while controlling stripe domain instability and enhancing their thermal stability. The trained DRL agent discovers an optimized field-temperature path that achieves a higher success rate for skyrmion formation in Fe3GeTe2 monolayers compared to previous fixed-temperature field sweeps. Additionally, the generated skyrmions exhibit longer lifetimes due to their isotropic shape, which tends to suppress internal excitation modes associated with skyrmion annihilation. We demonstrate that these advancements stem from the targeted minimization of the dissipated work, which ensures that the driven skyrmion states remain close to their equilibrium distributions by upper-bounding the Kullback-Leibler divergence. Our findings suggest that a DRL-powered search streamlines the identification of optimized protocols for skyrmion creation and control.
Surface acoustic waves (SAWs) become a popular driving source in modern condensed matter physics, but most existing theories simplify them as electric fields and ignore the non-uniform Brillouin zone folding effect. We develop a semiclassical framework and reconstruct the electron dynamics by treating SAW as a quasi-periodic potential modulating electronic momentum distribution. This framework naturally explains the experimentally observed DC drag current and predicts acousto-electric Hall effect. The theory further reveals various SAW-driven transport phenomena, emerging anomalous Hall, thermal Hall, and Nernst effects within time-reversal symmetric systems. Illustrated in bilayer graphene and $\mathrm{MX_2}$ (M = Mo, W; X = S, Se, Te), the angular-dependent acousto-electric Hall effect provides an experimental probe for Berry curvature distribution.
Nonlinear Hall responses are a direct electrical probe of quantum geometry, but they are symmetry-forbidden in many pristine two-dimensional metals. We show that layer-selective magnetic proximity unlocks intrinsic linear and nonlinear Hall effects in metallic $1H-NbX_2$ ($X=\mathrm{S,Se,Te}$), where native $D_{3h}$ symmetry forces both the anomalous Hall conductivity and the Berry-curvature dipole (BCD) to vanish. Fully relativistic density-functional theory combined with Wannier interpolation reveals that an out-of-plane proximity exchange that preserves $C_3$ generates a sizable sheet anomalous Hall conductivity, $σ^{\mathrm{sheet}}_{xy} \sim 10^{-2}(e^2/h)$, while keeping the BCD exactly zero. Breaking $C_3$ by adding an in-plane exchange component (or an orthogonal two-sided exchange texture) produces a strongly tunable BCD and hence a nonlinear Hall conductivity that is odd and approximately linear in the in-plane exchange scale, reaching $|D_y|$ of order $10^{-2}$ angstrom and maximized in NbTe$_2$. These magnitudes imply a readily measurable second-harmonic Hall voltage in micron-scale Hall bars under mA ac drive. We further propose a dual-interface device in which the signs of the first- and second-harmonic Hall voltages provide two-bit readout using the same contacts.
The energy spectrum and wave functions of electrons in a single silicon quantum dot provide valuable insights into the capabilities and limitations of such a system in quantum information processing. Here we investigate the low-lying singlet and triplet configurations and spectra in a two-electron silicon quantum dot. To build toward a comprehensive understanding, we first examine the competition between Coulomb interaction and electron kinetic and confinement energy in the absence of valley-orbit coupling, as well as consequences of valley blockade in the presence of an ideal smooth interface. For realistic interfaces the variations in the magnitude and phase of valley-orbit coupling lead to inter-valley leakage, particularly when orbital splittings approach the valley splitting. In our study we particularly focus on the impact on the compositions of low-lying singlets and triplets. We find that for experimentally relevant parameter regimes the ground singlet and triplet states usually contain multiple configurations with significant weights as a result of a complicated competition among valley-orbit coupling, confinement potential, and Coulomb interaction. We further analyze the effects of an out-of-plane magnetic field on these the two-electron spectra. Our findings could have important implications for spin qubits in Si quantum dot in various contexts, such as qubit encoding and spin measurement.
Higher-order symmetric $X$-wave magnets consist of two groups. One includes $d$-wave, $g$-wave and $i$-wave altermagnets, while the other includes $p$-wave and $f$-wave odd-parity magnets. Recently, the possibility of $h$-wave magnets has been discussed. Motivated by this development, we systematically construct an $X$-wave magnet with $\left( N_{X}+1\right) $ nodes in three dimensions from an $X$-wave magnet with $N_{X}$ nodes in two dimensions by means of a dimensional extension, where $N_X=1,2,3,4,6$ for $X=p,d,f,g,i$, respectively. Based on this method, we predict $j$-wave magnets in three dimensions. Then, we argue how to identify each of these $X$-wave magnets experimentally. We show that the $X$-wave magnet is completely identified by measuring the nonlinear spin currents. In particular, we predict that there are no spin currents other than the fourth-order ones such as $σ_{\text{spin}}^{x^{3}y;z}$ in $h$-wave odd-parity magnets in three dimensions and the sixth-order ones such as $σ_{\text{spin}}^{x^{5}y;z}$ in $j$-wave odd-parity magnets in three dimensions. They function as spin-current diodes because the spin current exhibits unidirectional flow independent of the applied electric field.
The thermal relaxation problem between two parallel plates with the same temperature is investigated, aiming to study the behavior of the free energy of the dense gas described by the Enskog equation. Two types of Enskog equation have been used: one is the Enskog equation with the original Enskog factor, while the other is that with a modified Enskog factor proposed recently in Takata & Takahashi, Phys. Rev. E 111, 065108 (2025). The evaluated free energy is a natural extension of the thermodynamic free energy to the non-equilibrium state. It is observed that this free energy monotonically decreases in time for the modified factor version, while it is not necessarily the case for the original version. Differences are also observed in other quantities in their time evolutions, most typically in the density profile.
Mixed quantum-classical models are widely used to reduce the computational cost of fully quantum simulations. However, their general applicability across different classes of problems remains an open question. Here, we address this issue for systems featuring spin-orbit coupling. In particular, we study the interaction dynamics of quantum spin-1/2 and classical orbital momentum in one-dimensional models of Rashba nanowires. We tackle this problem by resorting to a new quantum-classical Hamiltonian model that, unlike conventional approaches, retains the Heisenberg principle and captures correlation effects beyond the common Ehrenfest approach. Based on Koopman wavefunctions in classical mechanics, the new model was recently implemented numerically via a particle scheme -- the koopmon method -- which is extended here to treat spin-orbit coupling. We apply the koopmon method to study the quantum-classical dynamics of nanowire models, with and without the presence of a harmonic potential and in both Rashba-dominated (strong coupling) and Zeeman-dominated (weak coupling) regimes. Considering realistic semiconductor parameters, the results are contrasted with both fully quantum and quantum-classical Ehrenfest dynamics. In the absence of external potential, the koopmon method qualitatively reproduces the features of the fully quantum evolution for all coupling regimes. While it exhibits a slight loss in spin accuracy compared to Ehrenfest simulations, the latter fail to capture the orbital dynamics. In the presence of a harmonic potential, the koopmon scheme reproduces the full quantum results with accuracy levels that are unachievable by the Ehrenfest model in both quantum and classical sectors. We conclude by presenting a test case that exhibits the formation of cat-like states.
The search for carbon-based materials with tailored dimensionality and properties remains an important topic in materials science, particularly for applications in electronics, photonics, and nanomechanics. Among the emerging platforms in this context, graphyne (GY) represents a class of two-dimensional (2D) carbon allotropes composed of benzene rings connected by acetylenic linkages, yielding networks containing both $sp$- and $sp^2$-hybridized carbon atoms. By analogy with the transformation of $sp^2$ carbon networks such as graphene into $sp^3$-bonded diamond through interlayer covalent bonding, we construct three-dimensional (3D) GY-derived frameworks (3DGY) by covalently connecting stacked $α$-, $β$-, and $γ$-GY sheets via out-of-plane acetylene bridges. This approach converts the original $sp^2$ nodes into $sp^3$ centers while preserving the $sp$ character of the acetylenic segments, producing fully $sp$-$sp^3$ carbon networks. Structural relaxation shows that the $α$-derived framework does not converge to a stable configuration within this scheme, whereas the $β$- and $γ$-3DGY phases form stable architectures. Density functional theory (DFT) calculations, combined with ab initio molecular dynamics (AIMD) simulations, confirm the energetic, thermal, and dynamical stability of these two systems and are further used to investigate their structural, mechanical, electronic, and optical properties. Mechanical analysis reveals anisotropic elastic behavior, whereas electronic structure calculations show indirect band gaps of approximately 0.15 eV for $β$-3DGY and 1.65 eV for γ-3DGY. Optical calculations further reveal anisotropic responses, with absorption extending from the infrared to the visible. These results identify β-3DGY and γ-3DGY as new three-dimensional carbon allotropes with distinct mechanical, electronic, and optical properties.
The deterministic realization of quantum light sources operating at telecom wavelengths is essential for long-distance fiber-based quantum communication and distributed quantum computing. In this work, we demonstrate that telecom O-band emission can be achieved from site-controlled InGaAs/GaAs quantum dots (QDs). Our concept utilizes a buried AlAs/Al$_2$O$_3$ stressor layer with the unique feature that induces a well-defined and controllable tensile strain field at the growth surface, enabling both a redshift of QD emission to the $\sim$1.3~μm range and site-selective nucleation at the mesa centers. This concept eliminates not only the need for strain-reducing layers (SRLs), which are known to degrade optical coherence, but also provides spatial control and spectral tunability. The grown telecom QDs show pure single-photon emission with $g^{(2)}(τ) = (5.0 \pm 1.0) \times 10^{-2}$ at 4 K and $(2.8 \pm 0.3) \times 10^{-1}$ at 77~K, demonstrating the quantum nature and thermal stability of the emitters. The emission characteristics of complex excitonic states are analyzed using 8-band $k \cdot p$ and configuration-interaction modeling, which quantitatively reproduces the experimental observations. Finally, we present a theory-supported strategy to further redshift the emission toward the center of the O-band and beyond by employing a multi-buried-stressor approach. This combined framework of experiment and theory establishes the buried stressor concept as a scalable route toward highly coherent, position-controlled O-band quantum emitters compatible with industrial photonic integration.
We investigate the Goos--Hänchen (GH) shifts and group delay time of Dirac fermions traversing a rectangular electrostatic potential barrier in silicene. By analyzing their dependence on the incident angle, barrier height, barrier width, and incident energy, we demonstrate that the GH shifts exhibit pronounced oscillations arising from quantum interference within the barrier region. The amplitude and number of oscillation peaks increase with increasing energy, barrier width, and incidence angle, resulting in enhanced lateral beam displacement. Meanwhile, the group delay time exhibits resonant features associated with the formation of quasi-bound states, increasing with barrier width, energy, and incidence angle, while decreasing with increasing barrier height. These results clarify how barrier-induced quantum interference controls both the lateral and temporal dynamics of Dirac fermions in silicene, highlighting the potential role of electrostatic barriers in enabling tunable transport in two-dimensional Dirac materials.
Altermagnets have recently emerged as a new platform for spintronics applications, offering spin-split electronic bands despite vanishing net magnetization. Here, we investigate spin-current generation in Dirac altermagnets and identify Klein tunneling as an efficient mechanism for enhancing spin transport. Using a low-energy Dirac model combined with scattering theory, we demonstrate that Klein tunneling in altermagnets is strongly spin-dependent and can be used to effectively control the electronic spin-current polarization by, for instance, adjusting the height, width and orientation of the potential barrier. Finally, we explore how the l-wave symmetry of the Dirac altermagnet shapes the spin-current polarization and transmission, focusing especially on the d- and g-wave cases. Particularly promising results are obtained for the g-wave Dirac altermagnet, as it is found that the presence of a potential barrier can significantly boost the spin-current polarization, even when the intrinsic polarization due to the spin-split band structure is vanishingly small. For a barrier implemented via electrostatic gating, such a mechanism would in turn allow the spin-current polarization to be switched on and off via a gate voltage.
Moiré superlattices have emerged as a premier platform for simulating the Hubbard model, yet achieving high tunability in square-lattice systems remains a key challenge. We demonstrate that $Γ$-valley twisted square homobilayers provide a faithful and highly tunable realization of $t-t'-U$ Hubbard model, extending the recent proposal in M-valley systems. We show that at small twist angles, an emergent layer-exchange symmetry decouples electronic states into flat bands residing on two nested square sublattices. An interlayer displacement field breaks this symmetry to induce controllable inter-sublattice hybridization, enabling wide-range experimental tuning of the effective hopping ratio $t'/t$. By establishing a direct correspondence between $Γ$- and M-valley systems, we provide a unified framework for understanding displacement-field tunability in square moiré physics. These findings establish $Γ$-valley twisted bilayers as a versatile platform for simulating the square-lattice Hubbard model and exploring its rich landscape of correlated phenomena.
Cavity exciton--polaritons are quasiparticles that form when quantum well excitons hybridize with a cavity mode. Here, we carry out photon correlation measurements under continuous wave resonant laser excitation to demonstrate quantum correlations between cavity--polaritons. Our experiments reveal an unexpectedly strong dependence of polariton interactions on cavity--exciton detuning. When the polaritons are predominantly exciton-like, we observe a transition from photon antibunching to bunching as the laser is tuned across the polariton resonance, in agreement with a simple Kerr-nonlinearity model. When the lower-branch polariton energy is tuned to induce a two-polariton Feshbach resonance with the biexciton mode, the degree of polariton antibunching becomes independent of the laser detuning: we explain our finding by invoking a dissipative blockade mechanism arising from large biexciton broadening. Our experiments demonstrate that the strong polariton blockade regime would be achieved by reducing the polariton decay rate by a factor of 10.