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Stabilization of premixed NH3/H2/air flames via bluff-body flame holders

Lukas Gaipl, Wei Guan, Ganesh Guggilla, Alexey Kropman, Frank Beyrau, Dominique Thévenin

Abstract

The stabilization mechanisms of fully premixed NH3/H2/air flames anchored behind a bluff body are investigated using combined experiments and direct numerical simulations. Particular attention is given to the interplay between preferential diffusion, heat release, flow recirculation, and turbulence-flame interaction. Comparison between non-reactive and reactive cases shows that thermal expansion strongly alters the flow field, increasing the recirculation zone length by about 40% and the shear layer width by roughly 50% near the end of the recirculation region. Excellent agreement between measurements and simulations for mean and fluctuating axial velocities validates the numerical approach. Analysis of the flame structure reveals a distinctive stabilization mechanism at the flame root: preferential hydrogen diffusion generates a localized diffusion flame branch that enhances radical production and promotes robust anchoring. Combustion proceeds sequentially, with hydrogen mainly consumed in the shear layer, followed by ammonia cracking and the main heat-release region. Near the bluff body, heat release is concentrated within the recirculation zone, while downstream regions are increasingly influenced by turbulence and velocity fluctuations. The roles of curvature and strain are quantified to assess stretch effects along the flame front. Convex curvature near the flame root enhances hydrogen enrichment and locally increases burning rates, reinforcing stabilization. In contrast, concave curvature and higher stretch near the end of the recirculation zone weaken the flame and mark a transition toward a turbulence-dominated regime. Overall, stabilization results from a coupled feedback between recirculation-driven heat exchange and rapid hydrogen oxidation, sustaining an intermediate ammonia reaction zone and enabling robust anchoring of carbon-free NH3/H2 flames.

Stabilization of premixed NH3/H2/air flames via bluff-body flame holders

Abstract

The stabilization mechanisms of fully premixed NH3/H2/air flames anchored behind a bluff body are investigated using combined experiments and direct numerical simulations. Particular attention is given to the interplay between preferential diffusion, heat release, flow recirculation, and turbulence-flame interaction. Comparison between non-reactive and reactive cases shows that thermal expansion strongly alters the flow field, increasing the recirculation zone length by about 40% and the shear layer width by roughly 50% near the end of the recirculation region. Excellent agreement between measurements and simulations for mean and fluctuating axial velocities validates the numerical approach. Analysis of the flame structure reveals a distinctive stabilization mechanism at the flame root: preferential hydrogen diffusion generates a localized diffusion flame branch that enhances radical production and promotes robust anchoring. Combustion proceeds sequentially, with hydrogen mainly consumed in the shear layer, followed by ammonia cracking and the main heat-release region. Near the bluff body, heat release is concentrated within the recirculation zone, while downstream regions are increasingly influenced by turbulence and velocity fluctuations. The roles of curvature and strain are quantified to assess stretch effects along the flame front. Convex curvature near the flame root enhances hydrogen enrichment and locally increases burning rates, reinforcing stabilization. In contrast, concave curvature and higher stretch near the end of the recirculation zone weaken the flame and mark a transition toward a turbulence-dominated regime. Overall, stabilization results from a coupled feedback between recirculation-driven heat exchange and rapid hydrogen oxidation, sustaining an intermediate ammonia reaction zone and enabling robust anchoring of carbon-free NH3/H2 flames.
Paper Structure (7 sections, 4 equations, 12 figures, 1 table)

This paper contains 7 sections, 4 equations, 12 figures, 1 table.

Figures (12)

  • Figure 1: Geometry and boundary conditions.
  • Figure 2: Experimental setup and measurement arrangement.
  • Figure 3: Comparison of experimental (left) and numerical (right) axial velocity fields for the reactive case.
  • Figure 4: Axial velocity normalized by annular velocity (Tab. \ref{['tab:Conditions']}) on a central line through the bluff-body for experiments and simulations. Axial velocity is normalized by the annular velocity ($U=4.31$ m/s) and downstream distance by the bluff-body diameter ($D_{BB}=15$ mm).
  • Figure 5: Axial mean velocity comparison for increasing downstream distances from left to right, normalized by the experimental recirculation zone length ($L_{RZ}$). Velocities are normalized by the annular velocity $U$(Tab. \ref{['tab:Conditions']}).
  • ...and 7 more figures