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Control of helix orientation in chiral magnets via lateral confinement

Maurice Colling, Mariia Stepanova, Mario Hentschel, Somasree Bhattacharjee, Erik Lysne, Kasper Hunnestad, Naoya Kanazawa, Yoshinori Tokura, Jan Masell, Dennis Meier

TL;DR

This work demonstrates that lateral confinement in a DMI-driven helimagnet (FeGe) induces a chiral surface twist that acts as an effective surface anisotropy, governing the in-plane orientation of the helix propagation vector $\bm{q}$ in confined geometries. The authors develop an analytical boundary-condition–based model and validate it with micromagnetic simulations and MFM experiments on FeGe nanostructures, showing that $\bm{q}$ reorients continuously with aspect ratio and matches predictions for large systems. The results establish geometry-induced anisotropy as a general mechanism to steer DMI-stabilized spin-spiral states, with direct implications for device-level control in helimagnets and potential extensions to multilayers and synthetic chiral heterostructures.

Abstract

Helimagnetic materials offer a versatile platform for spin-based device concepts owing to their long-range, tunable spiral order. Here, we demonstrate controlled manipulation of the helimagnetic propagation vector q by geometrical confinement, using FeGe as a model DMI-driven chiral magnet. Micromagnetic simulations based on the nonlinear sigma model reveal that open boundaries give rise to a chiral surface twist acting as an effective surface anisotropy, which dictates the preferred helix orientation in the absence of magnetostatic shape effects. This geometry-induced anisotropy is quantitatively captured by an analytical model derived from the DMI boundary condition. Magnetic force microscopy measurements on focused-ion-beam structured FeGe confirm the predicted orientation behavior and establish geometry-controlled helimagnetic order as a robust, tunable mechanism for steering DMI-stabilized spin-spiral states. The concept provides a general route toward device-level control of chiral magnetic order in of non-centrosymmetric systems.

Control of helix orientation in chiral magnets via lateral confinement

TL;DR

This work demonstrates that lateral confinement in a DMI-driven helimagnet (FeGe) induces a chiral surface twist that acts as an effective surface anisotropy, governing the in-plane orientation of the helix propagation vector in confined geometries. The authors develop an analytical boundary-condition–based model and validate it with micromagnetic simulations and MFM experiments on FeGe nanostructures, showing that reorients continuously with aspect ratio and matches predictions for large systems. The results establish geometry-induced anisotropy as a general mechanism to steer DMI-stabilized spin-spiral states, with direct implications for device-level control in helimagnets and potential extensions to multilayers and synthetic chiral heterostructures.

Abstract

Helimagnetic materials offer a versatile platform for spin-based device concepts owing to their long-range, tunable spiral order. Here, we demonstrate controlled manipulation of the helimagnetic propagation vector q by geometrical confinement, using FeGe as a model DMI-driven chiral magnet. Micromagnetic simulations based on the nonlinear sigma model reveal that open boundaries give rise to a chiral surface twist acting as an effective surface anisotropy, which dictates the preferred helix orientation in the absence of magnetostatic shape effects. This geometry-induced anisotropy is quantitatively captured by an analytical model derived from the DMI boundary condition. Magnetic force microscopy measurements on focused-ion-beam structured FeGe confirm the predicted orientation behavior and establish geometry-controlled helimagnetic order as a robust, tunable mechanism for steering DMI-stabilized spin-spiral states. The concept provides a general route toward device-level control of chiral magnetic order in of non-centrosymmetric systems.
Paper Structure (14 sections, 4 equations, 5 figures)

This paper contains 14 sections, 4 equations, 5 figures.

Figures (5)

  • Figure 1: Helical spin order in FeGe. (a) Schematic illustration of the helical ground state showing the wavelength $\lambda$ and propagation direction $\bm{q}$. (b) Micromagnetic simulation of the helical state with the magnetization shown as arrows and color-coded according to the local magnetization direction (black = down, white = up, red = right, cyan = left). (c) Corresponding color-map representation of the same state as in (b).
  • Figure 2: Shape anisotropy in a rectangular magnet with an aspect ratio of 2:1. (a) Simulated ferromagnetic state including dipolar interactions, showing alignment of $\bm{M}$ along the long axis due to conventional shape anisotropy. (b) Simulated helical state without demagnetization energy, where the propagation vector $\bm{q}$ aligns diagonally to minimize the boundary energy through the chiral surface twist. (c) Corresponding energy landscapes as a function of orientation angle $\theta$. Orange stars mark the energy minima. The inset shows the calculated surface-twist contribution.
  • Figure 3: Dependence of the helix orientation on the aspect ratio of the confined region. (a) Color-coded phase diagram of the equilibrium orientation angle $\theta$ between $\bm{q}$ and $\hat{e}_x$, plotted as a function of lateral dimensions $L_x$ and $L_y$. Blue and red correspond to $\theta=0^{\circ}$ and $90^{\circ}$, respectively. Black squares mark data points for which the corresponding real-space textures are shown in (b). (b) Representative relaxed helical states for selected aspect ratios. (c) Orientation angle $\theta$ as a function of the aspect ratio $L_x/L_y$. Dots show numerical results colored by the total circumference; the black line represents the analytical model derived from the DMI boundary condition. Dashed segments denote the range outside the model’s validity ($6^{\circ} \lesssim\theta \lesssim 84^{\circ}$). The inset illustrates the restricted Fourier transform used to extract $\theta$, shown here for $(L_x,L_y) = (10.5\lambda,2.5\lambda)$, corresponding to the orange box in panels (a,b).
  • Figure 4: Experimental observation of helimagnetic order under lateral confinement. (a) SEM image of a 1 µ m thick FeGe lamella with an aspect ratio of approximately 1:2. (b) Corresponding MFM image revealing helimagnetic order, with propagation vector $\bm{q}$ tilted relative to the long axis. (c) Fast Fourier transform (FFT) of the MFM image used to determine the orientation angle $\theta$ between $\bm{q}$ and the long axis, yielding $23.7 \pm 1.4^{\circ}$.
  • Figure 5: Influence of lateral confinement on the helix orientation. (a–c) SEM images of rectangular FIB-cut regions with aspect ratios of about 1:1, 2:1, and 7:1, respectively. Overlaid MFM scans show the corresponding helimagnetic stripe patterns. White arrows indicate the direction of the helical propagation vector $\bm{q}$ inside each confined region, and the extracted orientation angle $\theta$ relative to the long side of the rectangle. The comparison between interior and exterior orientations demonstrates the predictable geometry-dependent reorientation of $\bm{q}$ in agreement with simulation results.