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The throttling refrigeration system for the large cooling power recovery of the PandaX-xT cryogenic distillation system for radon removal

Shunyu Yao, Zhou Wang, Kangkang Zhao, Zhi Zheng, Haoyu Wang, Xiangyi Cui, Tao Zhang, Li Zhao, Huaikuang Ding, Wenbing Tao, Xiang Xiao, Shaobo Wang, Yonglin Ju, Jianglai Liu, Xiangdong Ji, Shuaijie Li, Manbin Shen, Chengbo Du

TL;DR

The paper tackles the challenge of supplying a large, continuous cooling power for PandaX-xT's radon-removal cryogenic distillation, proposing an $\mathrm{R14}$-based throttling refrigeration system that transfers latent heat between the reboiler and the LXe cryostat to create a closed cooling cycle. The authors validate the concept with an ethanol-based R&D setup, achieving $Q\approx 17\ \mathrm{kW}$ at $\eta\approx 76.5\%$ and demonstrating substantial potential LN2 and power savings, while also modeling the system in Aspen Hysys with a deviation of $<2.5\%$ from experiments. Process simulations using the Peng-Robinson EOS are used to understand parameter sensitivities and to identify operating conditions that maximize efficiency, with an optimal scenario reaching $\eta_{\mathrm{opt}}=93.07\%$. The work provides a practical, energy-efficient solution for high-flow LXe distillation and radon removal, offering design guidance for future large-scale cryogenic systems and reducing dependence on LN2 and cryocoolers. The combination of experimental validation and rigorous simulation supports the viability and scalability of large cooling power recovery in cryogenic distillation contexts.

Abstract

In order to solve the continuous large cooling power supply problem (20 kW) for the radon-removal cryogenic distillation system, which operates at high liquid ffow rate of 856 kg/h (5 LPM) for the dark matter detector PandaX-xT of the next-generation, a throttling refrigeration system based on carbon tetraffuoride (R14) refrigerant for cooling power recovery is designed and developed. According to this system, the cooling power of the liquid xenon in the reboiler of 178K could be transferred to the product xenon cryostat to liquefy the gaseous product xenon by the R14 circulation, thus the liqueffed xenon could return to the detector with the same condition of which extracted from the detector to form a stable cooling cycle and prevent the instability of the detector. A research and development experiment is implemented to validate the feasibility of this large cooling recovery system, using the ethanol to simulate the liquid xenon. Experimental results show that the cooling power recovery of this system could achieve 17 kW with the efffciency of 76.5%, and the R14 ffow rate is 0.16 kg/s. This study realizes the online radon removal distillation with large ffow rate while eliminating the dependence of liquid nitrogen or cryocoolers, which means saving 2414 m3 liquid nitrogen per year or the power consumption of 230 kW. Furthermore, process simulation and optimization of the throttling refrigeration cycle is studied using Aspen Hysys to reveal the inffuences of the key parameters to the system, and the deviation between the simulation and experimental results is < 2.52%.

The throttling refrigeration system for the large cooling power recovery of the PandaX-xT cryogenic distillation system for radon removal

TL;DR

The paper tackles the challenge of supplying a large, continuous cooling power for PandaX-xT's radon-removal cryogenic distillation, proposing an -based throttling refrigeration system that transfers latent heat between the reboiler and the LXe cryostat to create a closed cooling cycle. The authors validate the concept with an ethanol-based R&D setup, achieving at and demonstrating substantial potential LN2 and power savings, while also modeling the system in Aspen Hysys with a deviation of from experiments. Process simulations using the Peng-Robinson EOS are used to understand parameter sensitivities and to identify operating conditions that maximize efficiency, with an optimal scenario reaching . The work provides a practical, energy-efficient solution for high-flow LXe distillation and radon removal, offering design guidance for future large-scale cryogenic systems and reducing dependence on LN2 and cryocoolers. The combination of experimental validation and rigorous simulation supports the viability and scalability of large cooling power recovery in cryogenic distillation contexts.

Abstract

In order to solve the continuous large cooling power supply problem (20 kW) for the radon-removal cryogenic distillation system, which operates at high liquid ffow rate of 856 kg/h (5 LPM) for the dark matter detector PandaX-xT of the next-generation, a throttling refrigeration system based on carbon tetraffuoride (R14) refrigerant for cooling power recovery is designed and developed. According to this system, the cooling power of the liquid xenon in the reboiler of 178K could be transferred to the product xenon cryostat to liquefy the gaseous product xenon by the R14 circulation, thus the liqueffed xenon could return to the detector with the same condition of which extracted from the detector to form a stable cooling cycle and prevent the instability of the detector. A research and development experiment is implemented to validate the feasibility of this large cooling recovery system, using the ethanol to simulate the liquid xenon. Experimental results show that the cooling power recovery of this system could achieve 17 kW with the efffciency of 76.5%, and the R14 ffow rate is 0.16 kg/s. This study realizes the online radon removal distillation with large ffow rate while eliminating the dependence of liquid nitrogen or cryocoolers, which means saving 2414 m3 liquid nitrogen per year or the power consumption of 230 kW. Furthermore, process simulation and optimization of the throttling refrigeration cycle is studied using Aspen Hysys to reveal the inffuences of the key parameters to the system, and the deviation between the simulation and experimental results is < 2.52%.
Paper Structure (18 sections, 15 equations, 16 figures, 1 table)

This paper contains 18 sections, 15 equations, 16 figures, 1 table.

Figures (16)

  • Figure 1: Diagram of the Rn-removal distillation with Xe loop and R14 loop
  • Figure 2: Large cooling power recovery throttling refrigeration flow diagram. 1. compressor outlet 2. reboiler inlet 3. reboiler outlet 4. LXe cryostat inlet 5. LXe cryostat outlet 6. compressor inlet.
  • Figure 3: Temperature-Entropy (T-S) diagram of the large cooling power recovery throttling refrigeration system, in which the black lines in the temperature-entropy diagram are isobaric lines to reflect the status of R14
  • Figure 4: R&D experiment flow diagram of the large cooling power recovery throttling refrigeration. In which T is the temperature measuring point and P is the pressure measuring point. 1.compressor outlet 2.simulated reboiler inlet 3.simulated reboiler outlet 4.simulated cryostat inlet 5.simulated cryostat outlet 6.compressor inlet.
  • Figure 5: (a) R&D experimental setup of the large cooling power recovery throttling refrigeration system (b) Compressor (c) Simulated reboiler heat exchanger and plate heat exchanger (d) Simulated cryostat heat exchanger (e) Throttle valve (f) R14 recycling system
  • ...and 11 more figures