Structures in higher-order quantum correlations due to non-spatial symmetries
Li Sun, Chong Chen, Ren-Bao Liu
TL;DR
This work reveals deep structures in higher-order quantum correlations arising from non-spatial symmetries. It derives generalized relations from time-translation invariance that constrain CTOCs and reduce the independent high-order Wightman correlations, and it establishes a framework to relate CTOCs to OTOCs via symmetry-induced mappings. The authors show that T- and S-symmetries connect OTOCs of different ranks, enabling access to certain rank-2 OTOCs through QNS without time-reversal, and they formulate a generalized fluctuation-dissipation theorem for higher-order correlations. Demonstrating with the transverse-field Ising model, they verify the selection rules, rank-conversion relations, and the higher-order FDT, highlighting practical paths to probe information scrambling through CTOCs.
Abstract
Quantum nonlinear spectroscopy (QNS) via a quantum sensor can access $2^{n-1}$ types of $n$-th order contour-time-ordered correlations (CTOCs) arising from different orderings of quantum operators, while classical nonlinear spectroscopy can detect only one in each order. QNS and its classical counterpart have similar spatial symmetry properties, but they are expected to have characteristically different non-spatial symmetry properties since different orderings of operators can behave differently under non-spatial transformations (such as exchange of operators). Here, we investigate how higher-order correlations extracted by QNS are constrained by non-spatial symmetries, including particle-hole (C), time-reversal (T), chiral (S) symmetry, and time translation symmetry. We find that the generalized C-symmetry imposes special selection rules on QNS, and the generalized T- and S-symmetry relate CTOCs to out-of-time-order correlations (OTOCs). The time translation symmetry leads to a generalized fluctuation-dissipation theorem for the spectra of higher-order CTOCs and OTOCs. This work discloses deep structures in higher-order quantum correlations due to non-spatial symmetries and provides access to certain types of OTOCs that are not directly observable.
