Dimensionality-induced dynamical phase transition in the large deviation of local time density for Brownian motion
Ruofei Yan, Hanshuang Chen
TL;DR
This work analyzes the large-deviation fluctuations of the local time density $\rho_T$ of a $d$-dimensional Brownian particle at a unit sphere, framing the problem through the tilted generator $\mathcal{L}_k=\nabla^2 + k\delta(r-1)$ and its dominant eigenvalue $\lambda(k)$. By solving the radial eigenproblem in terms of modified Bessel functions and enforcing proper boundary and matching conditions, the authors derive the SCGF $\lambda(k)$ and obtain the rate function $I(\rho)$ via the Legendre-Fenchel transform, uncovering a dimension-dependent dynamical phase transition. For $d\le 4$, $I(\rho)$ is analytic with a second-order singularity in $\lambda(k)$ at $k_c^{(d)}=d-2$ for $2<d\le 4$, while for $d>4$ a first-order transition appears with a linear branch $I(\rho)=(d-2)\rho$ for $0<\rho<\rho_c^{(d)}$ and $\rho_c^{(d)}=\frac{d(d-4)}{2d-4}$, signaling temporal phase separation in trajectory ensembles. The predictions are corroborated by rare-event simulations using multiple histogram reweighting, demonstrating the practical relevance of dimension-driven dynamical phase transitions in diffusion observables.
Abstract
We study the fluctuation properties of the local time density, ${ρ_T} = \frac{1}{T}\int_0^T {δ( {r(t) - 1} )} dt$, spent by a $d$-dimensional Brownian particle at a spherical shell of unit radius, where $r(t)$ denotes the radial distance from the particle to the origin. In the large observation time limit, $T \to \infty$, the local time density $ρ_T$ obeys the large deviation principle, $P(ρ_T= ρ) \sim e^{-T I(ρ)}$, where the rate function $I(ρ)$ is analytic everywhere for $d\leq 4$. In contrast, for $d>4$, $I(ρ)$ becomes nonanalytic at a specific point $ρ=ρ_c^{(d)}$, where $ρ_c^{(d)}=d(d-4)/(2d-4)$ depends solely on dimensionality. The singularity signals the occurrence of a first-order dynamical phase transition in dimensions higher than four. Such a transition is accompanied by temporal phase separations in the large deviations of Brownian trajectories. Finally, we validate our theoretical results using a rare-event simulation approach.
