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Granular segregation across flow geometries: a closure model for the particle segregation velocity

Yifei Duan, Lu Jing, Paul B. Umbanhowar, Julio M. Ottino, Richard M. Lueptow

TL;DR

This work delivers a general, first-principles closure for the segregation velocity $w_i$ in dense bidisperse granular flows by balancing the particle weight, a force of segregation $F^S_i$, and granular drag $F^D_i$, with diffusion corrections. By combining a gravity- and kinematics-enabled segregation force model with a Stokes-like drag law informed by $ ext{μ(I)}$ rheology and a volume-flux conservation constraint, the authors derive closed-form expressions for the species-specific segregation velocities in mixtures and demonstrate their validity against extensive DEM simulations across controlled and natural flow geometries. Incorporating diffusion through $D = A \\dot\gamma ar d^2$ yields net velocities that accurately capture segregation fluxes in inhomogeneous concentration fields. The framework, which can be embedded in the advection-diffusion-segregation equation, advances predictive capability for industrial and geophysical granular flows, while acknowledging current limitations in large-size-ratio, cohesive, and flow-coupled regimes and outlining clear paths for extension.

Abstract

Predicting particle segregation has remained challenging due to the lack of a general model for the segregation velocity that is applicable across a range of granular flow geometries. Here, a segregation velocity model for dense granular flows is developed by exploiting momentum balance and recent advances in particle-scale modelling of the segregation driving and drag forces over a wide range of particle concentrations, size and density ratios, and flow conditions. This model is shown to correctly predict particle segregation velocity in a diverse set of idealized and natural granular flow geometries simulated using the discrete element method. When incorporated in the well-established advection-diffusion-segregation formulation, the model has the potential to accurately capture segregation phenomena in many relevant industrial application and geophysical settings.

Granular segregation across flow geometries: a closure model for the particle segregation velocity

TL;DR

This work delivers a general, first-principles closure for the segregation velocity in dense bidisperse granular flows by balancing the particle weight, a force of segregation , and granular drag , with diffusion corrections. By combining a gravity- and kinematics-enabled segregation force model with a Stokes-like drag law informed by rheology and a volume-flux conservation constraint, the authors derive closed-form expressions for the species-specific segregation velocities in mixtures and demonstrate their validity against extensive DEM simulations across controlled and natural flow geometries. Incorporating diffusion through yields net velocities that accurately capture segregation fluxes in inhomogeneous concentration fields. The framework, which can be embedded in the advection-diffusion-segregation equation, advances predictive capability for industrial and geophysical granular flows, while acknowledging current limitations in large-size-ratio, cohesive, and flow-coupled regimes and outlining clear paths for extension.

Abstract

Predicting particle segregation has remained challenging due to the lack of a general model for the segregation velocity that is applicable across a range of granular flow geometries. Here, a segregation velocity model for dense granular flows is developed by exploiting momentum balance and recent advances in particle-scale modelling of the segregation driving and drag forces over a wide range of particle concentrations, size and density ratios, and flow conditions. This model is shown to correctly predict particle segregation velocity in a diverse set of idealized and natural granular flow geometries simulated using the discrete element method. When incorporated in the well-established advection-diffusion-segregation formulation, the model has the potential to accurately capture segregation phenomena in many relevant industrial application and geophysical settings.

Paper Structure

This paper contains 16 sections, 31 equations, 9 figures.

Figures (9)

  • Figure 1: (left) DEM simulation example of large (4 mm, blue) and small (2 mm, red) spheres in a uniform shear flow with downward gravity (negative $z$-direction), partitioned into 2.5$d_l$ high layers (shading) for characterizing depth-varying segregation velocity. Here, large particles rise while small particle sink. The segregation direction varies in the different flow configurations analyzed later. (right) Force balances on a large particle and a small particle corresponding to equation (\ref{['force_balance']}) and species-specific vertical segregation velocities, $w_i$.
  • Figure 2: (a) Large particle drag coefficient, $C^D_l$, vs. large particle species concentration, $c_l$, in a uniformly sheared flow for size ratios of $R_d=1.5$ at $I\approx 0.08$ (blue crosses) and $R_d=2$ at $I\approx 0.12$ (black circles) for $g=0$. Error bars show the standard deviation of $C^D_{l}$ over a 1 s window for $R_d=2$; error bars for $R_d=1.5$ are similar but omitted for clarity. Horizontal solid black line corresponds to $C^D_{i,0}$ for $R_d=2$; horizontal dashed blue line corresponds to $C^D_{i,0}$ for $R_d=1.5$. (b) Comparison of $C^D_{i,0}$ with $C^D_i$ for varying size ratio. The single intruder drag coefficient, $C^D_{i,0}$ is calculated from (\ref{['eq:drag_coefficient']}) for large ($i=l$ for $R_d\ge1$) (solid black curve) and small ($i=s$ for $R_d<1$) (dashed black curve) intruder particles. The mixture drag coefficient, $C^D_i$, (red curve) is calculated from (\ref{['eq:drag_coefficient']}) for $R_d\ge1$ and (\ref{['eq:conservation']}) for $R_d<1$. Both curves represent predictions for $I=0.2$. Predictions of the mixture model for $I$ values ranging from 0 (lower bound) to 0.4 (upper bound), which are typical of dense granular flows, are indicated by the shaded band.
  • Figure 3: Depth profiles (rows) of time averaged simulation results (symbols) and predictions (dashed black curves) for the four controlled shear flows (columns) in steady state at $R_d=2$. (a) Streamwise mean velocity $u$, (b) normalized segregation force on a large particle $\hat{F}^S_l=F^S_l/m_l g_0$, (c) bulk viscosity $\eta$, and (d) segregation velocity, $w_i$ for small (red) and large (blue) particles measured from the simulation (symbols) and predicted via (\ref{['eq:w']}) (curves). Dotted vertical lines in (b) indicate segregation force equal to particle weight. In all cases, $U=20\,$m s$^{-1}$, $c_l=c_s=0.5$, and $H\approx 0.2\,$m.
  • Figure 4: Profiles of the segregation velocity $w_i$ for large (blue) and small (red) particles with $R_d=2$ for the exponential velocity profile with $g=g_0$ and bulk large particle concentrations of (a) $c_l=0.2$, (b) $c_l=0.5$, and (c) $c_l=0.8$, based on the prescribed velocity profiles (solid curves) compared to DEM measurements (symbols) averaged over 1 s after the flow reaches steady state.
  • Figure 5: Effect of (a) three different spatially varying concentration profiles (columns) on the segregation velocity $w_i$ for (b) linear ($u=Uz/H$) and (c) exponential ($Ue^{k(z/H-1)}$) velocity profiles with $g=g_0$ and $R_d=2$. In rows (b) and (c), dashed curves represent model predictions using equation (\ref{['eq:w']}) for $w_i$, solid curves represent predictions corrected by the diffusion flux, i.e. $w^{net}_i$ from (\ref{['eq:w_net']}), and symbols indicate measurements from DEM simulations.
  • ...and 4 more figures